Auditable Human-Agent Teams for Autonomous X-ray Experimentation

arXiv:2611.12933v1 Announce Type: new Abstract: Closed-loop autonomous experimentation can accelerate scientific discovery, but implementation effort limits accessibility. Agentic systems may lower this barrier, although sustained operation on physical instruments remains largely unexplored. Here, using coding-agent infrastructure grounded in validated scientific methods, we demonstrate autonomous synchrotron X-ray experiments on nanoparticle superlattices under evolving, human-defined objectives. Complete human-agent and agent-agent transcripts enable an audit that reconstructs decision provenance and characterizes the division of cognitive labor.